By Gregory L. Geoffroy
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Wrighton, D . L. Morse, and L. Pdungsap, J. Am. Chem. Soc. 97, 2073 (1975). M. Wrighton, Η. B. Gray, and G. S. Hammond, Mol. Photochem. 5, 165 (1973). Y. S. Sohn, D . N . Hendrickson, and Η. B. Gray, J. Am. Chem. Soc. 93, 3603 (1970). M. S. Wrighton, D . I. Handeli, and D . L. Morse, Inorg. Chem. 15, 434 (1976); H. Haas and R. K. Sheline, J. Am. Chem. Soc. 88, 3219 (1966). J. C. D . Brand and W. Snedden, Trans. Faraday Soc. 53, 894 (1957). C. R. Bock and M. S. Wrighton, Inorg. Chem. 16, 1309 (1977).
The typical situation in organometallics is that the only detectable emission is that associated with the lowest excited state decaying to the ground state. Thus, the effective excitation wavelengths will be n o lower in energy than the emitted light, and quite naturally, only those exciting wavelengths which are effective in producing excited states will excite the emission. However, excitation wavelengths may directly produce upper excited states which m a y or may not decay to the lowest excited state from which emission occurs with a detectable yield.
M. S. Wrighton, Chem. Rev. 74, 401 (1974). Pure Appl. Chem. 28, 39 (1971). W. E. Silverthorn, Adv. Organomet. Chem. 13, 47 (1975). M. S. Wrighton, D . L. Morse, and L. Pdungsap, J. Am. Chem. Soc. 97, 2073 (1975). M. Wrighton, Η. B. Gray, and G. S. Hammond, Mol. Photochem. 5, 165 (1973). Y. S. Sohn, D . N . Hendrickson, and Η. B. Gray, J. Am. Chem. Soc. 93, 3603 (1970). M. S. Wrighton, D . I. Handeli, and D . L. Morse, Inorg. Chem. 15, 434 (1976); H. Haas and R. K. Sheline, J. Am. Chem. Soc. 88, 3219 (1966).